Force-detected nuclear double resonance between statistical spin polarizations

We demonstrate nuclear double resonance for nanometer-scale volumes of spins where random fluctuations rather than Boltzmann polarization dominate. When the Hartmann-Hahn condition is met in a cross-polarization experiment, flip-flops occur between two species of spins and their fluctuations become coupled. We use magnetic resonance force microscopy to measure this effect between 1H and 13C spins in 13C-enriched stearic acid. The development of a cross-polarization technique for statistical ensembles adds an important tool for generating chemical contrast in nanometer-scale magnetic resonance.Comment: 14 pages, 4 figure

Gate-controlled nuclear magnetic resonance in an AlGaAs/GaAs quantum Hall device

We study the resistively detected nuclear magnetic resonance (NMR) in an AlGaAs/GaAs quantum Hall device with a side gate. The strength of the hyperfine interaction between electron and nuclear spins is modulated by tuning a position of the two-dimensional electron systems with respect to the polarized nuclear spins using the side-gate voltages. The NMR frequency is systematically controlled by the gate-tuned technique in a semiconductor device.Comment: 3 pages, 4 figures, submitted to Appl. Phys. Let

Backscattering Between Helical Edge States via Dynamic Nuclear Polarization

We show that that the non-equilibrium spin polarization of one dimensional helical edge states at the boundary of a two dimensional topological insulator can dynamically induce a polarization of nuclei via the hyperfine interaction. When combined with a spatially inhomogeneous Rashba coupling, the steady state polarization of the nuclei produces backscattering between the topologically protected edge states leading to a reduction in the conductance which persists to zero temperature. We study these effects in both short and long edges, uncovering deviations from Ohmic transport at finite temperature and a current noise spectrum which may hold the fingerprints for experimental verification of the backscattering mechanism.Comment: 4+ pages, 4 figure

Soft-pulse dynamical decoupling in a cavity

Dynamical decoupling is a coherent control technique where the intrinsic and extrinsic couplings of a quantum system are effectively averaged out by application of specially designed driving fields (refocusing pulse sequences). This entails pumping energy into the system, which can be especially dangerous when it has sharp spectral features like a cavity mode close to resonance. In this work we show that such an effect can be avoided with properly constructed refocusing sequences. To this end we construct the average Hamiltonian expansion for the system evolution operator associated with a single ``soft'' pi-pulse. To second order in the pulse duration, we characterize a symmetric pulse shape by three parameters, two of which can be turned to zero by shaping. We express the effective Hamiltonians for several pulse sequences in terms of these parameters, and use the results to analyze the structure of error operators for controlled Jaynes-Cummings Hamiltonian. When errors are cancelled to second order, numerical simulations show excellent qubit fidelity with strongly-suppressed oscillator heating.Comment: 9pages, 5eps figure

Ferromagnetic Resonance in Spinor Dipolar Bose--Einstein Condensates

We used the Gross--Pitaevskii equations to investigate ferromagnetic resonance in spin-1 Bose--Einstein condensates with a magnetic dipole-dipole interaction. By introducing the dipole interaction, we obtained equations similar to the Kittel equations used to represent ferromagnetic resonance in condensed matter physics. These equations indicated that the ferromagnetic resonance originated from dipolar interaction, and that the resonance frequency depended upon the shape of the condensate. Furthermore, spin currents driven by spin diffusions are characteristic of this system.Comment: 8 pages, 10 figure

Optimized pulse sequences for suppressing unwanted transitions in quantum systems

We investigate the nature of the pulse sequence so that unwanted transitions in quantum systems can be inhibited optimally. For this purpose we show that the sequence of pulses proposed by Uhrig [Phys. Rev. Lett. \textbf{98}, 100504 (2007)] in the context of inhibition of environmental dephasing effects is optimal. We derive exact results for inhibiting the transitions and confirm the results numerically. We posit a very significant improvement by usage of the Uhrig sequence over an equidistant sequence in decoupling a quantum system from unwanted transitions. The physics of inhibition is the destructive interference between transition amplitudes before and after each pulse.Comment: 5 figure

Mixed state Pauli channel parameter estimation

The accuracy of any physical scheme used to estimate the parameter describing the strength of a single qubit Pauli channel can be quantified using standard techniques from quantum estimation theory. It is known that the optimal estimation scheme, with m channel invocations, uses initial states for the systems which are pure and unentangled and provides an uncertainty of O[1/m^(1/2)]. This protocol is analogous to a classical repetition and averaging scheme. We consider estimation schemes where the initial states available are not pure and compare a protocol involving quantum correlated states to independent state protocols analogous to classical repetition schemes. We show, that unlike the pure state case, the quantum correlated state protocol can yield greater estimation accuracy than any independent state protocol. We show that these gains persist even when the system states are separable and, in some cases, when quantum discord is absent after channel invocation. We describe the relevance of these protocols to nuclear magnetic resonance measurements

Unusual hyperfine interaction of Dirac electrons and NMR spectroscopy in graphene

Theory of nuclear magnetic resonance (NMR) in graphene is presented. The canonical form of the electron-nucleus hyperfine interaction is strongly modified by the linear electronic dispersion. The NMR shift and spin-lattice relaxation time are calculated as function of temperature, chemical potential, and magnetic field and three distinct regimes are identified: Fermi-, Dirac-gas, and extreme quantum limit behaviors. A critical spectrometer assessment shows that NMR is within reach for fully 13C enriched graphene of reasonable size.Comment: 5 pages, 3 figure

Optical pumping of quantum dot nuclear spins

An all-optical scheme to polarize nuclear spins in a single quantum dot is analyzed. The hyperfine interaction with randomly oriented nuclear spins presents a fundamental limit for electron spin coherence in a quantum dot; by cooling the nuclear spins, this decoherence mechanism could be suppressed. The proposed scheme is inspired by laser cooling methods of atomic physics and implements a "controlled Overhauser effect" in a zero-dimensional structure

Lower bound for electron spin entanglement from beamsplitter current correlations

We determine a lower bound for the entanglement of pairs of electron spins injected into a mesoscopic conductor. The bound can be expressed in terms of experimentally accessible quantities, the zero-frequency current correlators (shot noise power or cross-correlators) after transmission through an electronic beam splitter. The effect of spin relaxation (T_1 processes) and decoherence (T_2 processes) during the ballistic coherent transmission of the carriers in the wires is taken into account within Bloch theory. The presence of a variable inhomogeneous magnetic field allows the determination of a useful lower bound for the entanglement of arbitrary entangled states. The decrease in entanglement due to thermally mixed states is studied. Both the entanglement of the output of a source (entangler) and the relaxation (T_1) and decoherence (T_2) times can be determined.Comment: 4 pages, 3 figure